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Article Dans Une Revue Chemistry - A European Journal Année : 2020

Recyclable Ruthenium Catalyst for Distal meta ‐C−H Activation

Résumé

We disclose the unprecedented hybrid-ruthenium catalysis for distal meta-C−H activation. The hybrid-ruthenium catalyst was recyclable, as was proven by various heterogeneity tests, and fully characterized with various microscopic and spectroscopic techniques, highlighting the physical and chemical stability. Thereby, the hybrid-ruthenium catalysis proved broadly applicable for meta-C−H alkylations of among others purine-based nucleosides and natural product conjugates. Additionally, its versatility was further reflected by meta-C−H activations through visible-light irradiation, as well as para-selective C−H activations.
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Origine : Publication financée par une institution

Dates et versions

hal-03121169 , version 1 (03-06-2022)

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Paternité - Pas d'utilisation commerciale

Identifiants

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Isaac Choi, Valentin Müller, Yanhui Wang, Kai Xue, Rositha Kuniyil, et al.. Recyclable Ruthenium Catalyst for Distal meta ‐C−H Activation. Chemistry - A European Journal, 2020, 26 (66), pp.15290-15297. ⟨10.1002/chem.202003622⟩. ⟨hal-03121169⟩
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